Piezoelectric Properties of Mn-modified Na0.5Bi2.5Nb2O9 for High Temperature Applications

doi:10.3724/SP.J.1077.2012.11660

Abstract

Abstract: Bismuth layer-structured ferroelectric ceramics Na_0.5Bi_2.5Nb₂O₉(NBN+xmol% MnCO₃, 0≤x≤10.0) were synthesized by traditional solid state reaction. The effects of Mn addition on the microstructure and electrical properties of ceramics were investigated in detail. The results showed that all the ceramic samples were single-phase ferroelectrics with high Curie points (T_c≥700℃). With the addition of MnCO₃, the mechanical quality factor, piezoelectric activity and electromechanical properties of Na_0.5Bi_2.5Nb₂O₉-based ceramics are enhanced significantly. Besides, the NBN+8.0mol% MnCO₃ ceramic exhibits the optimum electrical properties: tanδ=0.749%, d₃₃=20 pC/N, Q_m=3120, k_p=12.37%, kt=21.09%, Pr=7.01 μC/cm². After annealing at 700℃, the d₃₃ value of NBN+8.0mol% MnCO₃ ceramic remains 75%(~15 pC/N), which indicates that this ceramic is a promising material for high temperature applications.

Key words: piezoelectric ceramics, microstructure, electromechanical properties, ferroelectric properties; Na_{0. 5}Bi_2.5Nb₂O₉

CLC Number:

TQ174

JIANG Xiang-Ping, WEN Jia-Xin, CHEN-Chao, TU-Na, LI Xiao-Hong. Piezoelectric Properties of Mn-modified Na_0.5Bi_2.5Nb₂O₉ for High Temperature Applications[J]. Journal of Inorganic Materials, 2012, 27(8): 827-832.

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Piezoelectric Properties of Mn-modified Na_0.5Bi_2.5Nb₂O₉ for High Temperature Applications

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