Sintering Temperature Influence on the Dielectric and Piezoelectric Properties of Pb(Mn1/3Sb2/3)O3-PbZrO3-PbTiO3 Ceramics

Abstract

Abstract: The effects of sintering temperature on the microstructure and piezoelectric properties of
Pb(Mn_1/3Sb_2/3)O₃-PbZrO₃-PbTiO₃ (PMS-PZT) ceramic were investigated. Results show that the optimized properties of ε_r=1530,
d₃₃=374pC/N, K_p=0.6, tanδ=0.41%, Q_m=1250 can be obtained when the ceramic sintered at 1240℃ for 2h, which suit for high-power applications. Meanwhile, the ceramic also possesses
superior characteristics (ε_r=1370, d₃₃=348pC/N, K_p=0.57, tanδ=0.62% and Q_m=1620) for multilayer components and thick-film devices when it sintered at 1150℃.
Results also indicate that PMS-PZT ceramic can be sintered in a wide temperature range. High temperature microscope, SEM, TEM, and EDS
investigation confirm that PbO and Sb_₂O_₅ can form a liquid phase acting as a secondary phase on grain boundaries at lower sintering
temperature, and then enter the crystal lattice to form perovskite structure at higher sintering temperature.

Key words: PMS-PZT, piezoelectric, sintering temperature, liquid phase

CLC Number:

TQ174

ZHU Zhi-Gang,LI Bao-Shan,LI Guo-Rong,ZHANG Wang-Zhong,YIN Qing-Rui. Sintering Temperature Influence on the Dielectric and Piezoelectric Properties of Pb(Mn_1/3Sb_2/3)O₃-PbZrO₃-PbTiO₃ Ceramics[J]. Journal of Inorganic Materials.

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Sintering Temperature Influence on the Dielectric and Piezoelectric Properties of Pb(Mn_1/3Sb_2/3)O₃-PbZrO₃-PbTiO₃ Ceramics

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