二维MXene材料在新型薄膜太阳能电池技术中的研究进展

doi:10.15541/jim20230510

无机材料学报 ›› 2024, Vol. 39 ›› Issue (2): 215-224.DOI: 10.15541/jim20230510 CSTR: 32189.14.10.15541/jim20230510

所属专题：【信息功能】MAX层状材料、MXene及其他二维材料(202409)；【能源环境】太阳能电池(202409)

二维MXene材料在新型薄膜太阳能电池技术中的研究进展

费玲¹^,²(), 雷蕾¹^,², 汪德高¹^,²^,³()

1.中国科学院宁波材料技术与工程研究所, 先进能源材料工程实验室, 宁波 315201
2.中国科学院大学, 北京 100049
3.中国科学院宁波材料所前沿交叉科学研究中心, 宁波 315201

收稿日期:2023-11-02 修回日期:2023-12-15 出版日期:2023-12-25 网络出版日期:2023-12-25
通讯作者: 汪德高, 研究员. E-mail: wangdegao@nimte.ac.cn
作者简介:费玲(1995-), 女, 硕士. E-mail: feiling@nimte.ac.cn
基金资助:
国家自然科学基金(22106166);宁波市甬江引才工程;中国博士后科学基金(2022M723253)

Progress of Two-dimensional MXene in New-type Thin-film Solar Cells

FEI Ling¹^,²(), LEI Lei¹^,², WANG Degao¹^,²^,³()

1. Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology& Engineering, Chinese Academy of Sciences, Ningbo 315201, China
2. University of Chinese Academy of Sciences, Beijing 100049, China
3. Research Center for Advanced Interdisciplinary Sciences of Ningbo Materials Institute, Chinese Academy of Sciences, Ningbo 315201, China

Received:2023-11-02 Revised:2023-12-15 Published:2023-12-25 Online:2023-12-25
Contact: WANG Degao, professor. E-mail: wangdegao@nimte.ac.cn
About author:FEI Ling (1995-), female, Master. E-mail: feiling@nimte.ac.cn
Supported by:
National Natural Science Foundation of China(22106166);Yongjiang Innovative Individual Introduction of China;China Postdoctoral Science Foundation(2022M723253)

摘要/Abstract

摘要：

太阳能作为自然界中丰富的可持续清洁能源, 可以在解决当前能源短缺问题的同时有效减少因过度消耗化石燃料造成的环境污染问题。近年来, 第三代新型薄膜太阳能电池, 如染料敏化太阳能电池(DSSCs)和钙钛矿太阳能电池(PSCs)等, 凭借其原料丰富、制造成本低廉和光电性能良好等优点而受到广泛关注。然而, 新型薄膜太阳能电池器件的电荷传输性能和运行稳定性与正式商用的要求仍有一定差距。二维MXene材料具有比表面积高、表面官能团丰富、导电性优良、功函数可调和亲水性等优点, 已成为能源转换领域的研究热点。鉴于此, 本文在综述二维MXene材料的结构、光学和电学特性的基础上, 阐述了近些年二维MXene材料应用于新型薄膜太阳能电池的研究进展, 并重点探讨了二维MXene材料增强太阳能电池光电性能的机制。二维MXene材料可通过作为钙钛矿太阳能电池中钙钛矿层和电荷传输层的添加剂、修饰染料敏化太阳能电池的光电阳极和制备电极, 来调整能带对齐、降低功函数、拓宽吸光范围和形成“柱撑效应”, 有效改善器件的光吸收效率、载流子迁移率和电荷提取能力, 从而提升器件的光电性能和稳定性。最后, 结合目前的研究进展, 对二维MXene材料在新型薄膜太阳能电池技术中的发展前景及面临的挑战提出了建议。

关键词: MXene, 纳米材料, 太阳能电池, 光电性能, 能源, 专题评述

Abstract:

As renewable and sustainable clean energy, solar energy has the potential to address current energy shortage and reduce environmental pollution caused by fossil fuels consumption. In recent years, the third-generation thin-film solar cells, such as dye-sensitized solar cells (DSSCs) and perovskite solar cells (PSCs), have attracted widespread attention due to their low cost, abundant materials, and high photoelectric performance. However, these devices still face challenges in terms of charge transfer efficiency and operational stability for their commercialization. Two-dimensional (2D) MXene materials have emerged as promising candidates for improving the performance of thin-film solar cells due to their unique properties, including high specific surface area, rich surface functional groups, high conductivity, tunable work function, and hydrophilicity. This review summarizes the recent research progress of 2D MXene materials applied in new thin-film solar cells, focusing on the reaction mechanism that enhances the photoelectric performance of solar cells. Strategies such as using 2D MXene materials as additives for the perovskite layer and charge transport layer in PSCs, modifying the photoanode in DSSCs, and preparing varous electrodes, can effectively improve light absorption efficiency, carrier mobility, and charge extraction capability of the devices by adjusting band alignment, reducing work function, broadening the light absorption range, and creating a “pillar support effect”. As a result, the photoelectric performance and stability of the devices are enhanced. In conclusion, the perspectives highlights the current research progress and challenge faced by 2D MXene materials in novel thin-film solar cells.

Key words: MXene, nano-material, solar cell, photoelectric performance, energy, perspective

中图分类号:

TQ174

费玲, 雷蕾, 汪德高. 二维MXene材料在新型薄膜太阳能电池技术中的研究进展[J]. 无机材料学报, 2024, 39(2): 215-224.

FEI Ling, LEI Lei, WANG Degao. Progress of Two-dimensional MXene in New-type Thin-film Solar Cells[J]. Journal of Inorganic Materials, 2024, 39(2): 215-224.

图/表 9

图1 二维MXene基纳米材料的应用[13,15,18-19]

Fig. 1 Application of 2D MXene-based nanomaterials[13,15,18-19] (a) Ti3C2Tx//CNT-HQ hybrid supercapacitors[13]; (b) Schematic diagram of flexible biomimetic Ti3C2 MXene-based platform for extracellular superoxide biosensing[15]; (c) Schematic photocatalytic water splitting mechanism for Ti3C2@TiO2@MoS2 composites[18]; (d) Schematic photocatalytic CO2 reduction for 2D/2D heterojunction of ultrathin Ti3C2/Bi2WO6 nanosheets[19]

图2 MAX相选择性蚀刻A原子层制备MXene[24]

Fig. 2 Schematic illustration of two approaches to produce MXene by removal of A layers from MAX phases and related layered compounds[24] (1) MAX phase selectively etched in fluoride ion-containing acids; (2) MAX phase selectively etched in molten salts

图3 Ti3C2T2 MXene对低光子能量(a)和大光子能量(b)的吸收光谱图[35]

Fig. 3 Absorption spectra of Ti3C2T2 MXene for small (a) and large (b) range of photon energy[35]

图4 Mo2TiC2, Mo3C和Ti3C MXene的电子结构[43]

Fig. 4 Electronic structures of Mo2TiC2, Mo3C and Ti3C MXene[43] (a-i) Total and projected densities of states for OH-, O-, and F-terminated Mo2TiC2 (a-c), Mo3C2 (d-f), and Ti3C2 (g-i) MXenes

图5 表面官能团对MXenes功函数的调控[46]

Fig. 5 Surface functional groups which affect the work functions of MXenes[46]

图6 新型薄膜太阳能电池结构[16-17]

Fig. 6 Structures of novel thin-film solar cells[16-17] (a) Schematic representation of a DSSC used the MXene[16]; (b) Schematic representation of a PSC used the MXene[17]

图7 原始PSC和掺杂MXene的PSC的UPS谱图和费米能级[42]

Fig. 7 UPS curves and energy versus Fermi level of pristine and MXene-doped perovskite films[42] (a) UPS spectra in the valence band (VB) region; (b) Energy scheme for undoped and MXene-doped perovskite with respect to the EFermi. IE: Ionization energy; EVAC: Vacuum level; BE: Binding energy

图8 TiO2/Ti3C2Tx光阳极性能[52]

Fig. 8 Photovoltaic performance of TiO2/Ti3C2Tx photoanode[52] (a, b) J-V curves (a) and IPCE curves (b) of champion DSSCs based on the TiO2 photoanode or TiO2/Ti3C2Tx photoanode under 100 mW/cm2; (c) Plots of PCE against FF of reported Z907-based DSSCs; (d) J-V curves of champion DSSCs based on the TiO2 photoanode or TiO2/Ti3C2Tx photoanode under dim light with an intensity of ∼1.9 mW/cm2 (6000 lux)

图9 MoP/MoNiP2@Ti3C2、MoP/MoNiP2和Pt对电极的光电性能比较[57]

Fig. 9 Photoelectric properties of MoP/MoNiP2@Ti3C2, MoP/MoNiP2 and Pt counter electrodes[57] (a) Photocurrent density-voltage curves of DSSCs with various CEs; (b) Distribution of PCEs of the DSSCs assembled with the MoP/MoNiP2@Ti3C2-80% CE; CE: counter electrode; PCE: power conversion efficiency

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二维MXene材料在新型薄膜太阳能电池技术中的研究进展

Progress of Two-dimensional MXene in New-type Thin-film Solar Cells

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