Journal of Inorganic Materials ›› 2022, Vol. 37 ›› Issue (4): 445-451.DOI: 10.15541/jim20210270
Special Issue: 【能源环境】金属有机框架材料; 【能源环境】钙钛矿
• RESEARCH LETTER • Previous Articles Next Articles
ZHANG Guoqing1,2(), QIN Peng1(), HUANG Fuqiang1,2,3()
Received:
2021-04-26
Revised:
2021-06-29
Published:
2022-04-20
Online:
2021-07-12
Contact:
QIN Peng, associate professor. E-mail: qinpeng@mail.sic.ac.cn;About author:
ZHANG Guoqing (1992–), male, PhD candidate. E-mail: zgq201209@foxmail.com
Supported by:
CLC Number:
ZHANG Guoqing, QIN Peng, HUANG Fuqiang. Reversible Conversion between Space-confined Lead Ions and Perovskite Nanocrystals for Confidential Information Storage[J]. Journal of Inorganic Materials, 2022, 37(4): 445-451.
Fig. 1 Schematic diagram of in-situ growth of MAPbBr3 NCs from Pb-ZIF framework and optical images of Pb-ZIF (left under ambient light), and MAPbBr3 NCs@Pb-ZIF (right under UV light)
Fig. 2 (a) TEM image and (b) SAED pattern of Pb-ZIF powders SEM images of (c, d) Pb-ZIF and (e) MAPbBr3 NCs@Pb-ZIF powders, and (f) Elemental mappings of MAPbBr3 NCs@Pb-ZIF powder
Fig. 3 XPS spectra of Pb-ZIF and MAPbBr3 NCs@Pb-ZIF samples (a) Survey XPS spectra; (b) Pb4f XPS spectra (The offset of Pb 4f peaks marked by an arrow); (c) Br3d XPS spectra of Pb-ZIF and MAPbBr3 NCs@Pb-ZIF samples; (d) Br3d XPS spectrum of MAPbBr3 NCs@Pb-ZIF sample after etching
Fig. 4 (a) Absorption and (b) steady-state PL spectra of Pb-ZIF and MAPbBr3 NCs@Pb-ZIF samples; (c) PL decay kinetics of MAPbBr3 NCs@Pb-ZIF sample; (d) Schematic confidential information encryption and decryption process based on Pb-ZIF and MAPbBr3 NCs@Pb-ZIF; (e) Optical images of the printed Pb-ZIF and MAPbBr3 NCs@Pb-ZIF patterns under UV excitation
Fig. 5 SEM images of (a) pristine commercial paper, (b) commercial paper after printed with Pb-ZIF ink, (c) commercial paper with MAPbBr3 NCs@Pb-ZIF NCs, (d) representative information encryption and decryption procedure, and (e) PL intensity of the printed MAPbBr3 NCs@Pb-ZIF patterns in the five cycles of encryption and decryption measurement
Fig. S1 X-ray diffraction patterns of Pb-ZIF and MAPbBr3 NCs@Pb-ZIF powders The ideal diffraction peaks of MAPbBr3 were presented as red vertical line
Fig. S4 (a) UV-Vis absorption spectra of the printed Pb-ZIF and MAPbBr3 NCs@Pb-ZIF patterns, (b) steady-state PL spectra and (c) PL decay kinetics of the printed MAPbBr3 NCs@Pb-ZIF patterns
τ1/ns | f1 | τ2/ns | f2 | τavg/ns | |
---|---|---|---|---|---|
Powder | 4.0 | 82.7% | 16.3 | 17.3% | 6.1 |
Table S1 PL lifetime for MAPbBr3 NCs@Pb-ZIF powders
τ1/ns | f1 | τ2/ns | f2 | τavg/ns | |
---|---|---|---|---|---|
Powder | 4.0 | 82.7% | 16.3 | 17.3% | 6.1 |
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